4.3 Article

Mechanical properties and microstructure in neutron-irradiated nickel-based alloys and stainless steels for supercritical water-cooled-reactor fuel cladding

Journal

JOURNAL OF NUCLEAR SCIENCE AND TECHNOLOGY
Volume 57, Issue 1, Pages 114-120

Publisher

TAYLOR & FRANCIS LTD
DOI: 10.1080/00223131.2019.1660730

Keywords

Stainless steel; nickel alloy; neutron irradiation; tensile behavior; transmission-electron-microcopy observation; supercritical water reactor; precipitate

Funding

  1. Institute of Applied Energy (IAE), Ministry of Economy, Trade and Industry (METI), Japan
  2. Interuniversity Cooperative Research Program of International Research Center for Nuclear Materials Science, the Institute for Materials Research, Tohoku University [17M0016, 18M0019, 18K0082]

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To investigate the irradiation behavior of mechanical properties and microstructural changes of commercial Ni-based alloys and improved stainless steels, a neutron-irradiation experiment was performed at the Joyo reactor, and post-irradiation examinations with tensile tests and TEM observations were carried out. The room-temperature tensile tests showed that all specimens that were irradiated at 485 degrees C exhibited significant hardening and ductile behavior, especially in alloy 625. The irradiation hardening of all specimens irradiated at 668 degrees C was less than that of specimens irradiated at 485 degrees C. The fine-grained stainless steel, T3 and the Zr-added stainless steels, H1 and H2 showed good mechanical-property performance with keeping ductility after neutron irradiation. Most alloys and steels showed ductile behavior on the fracture surface except for alloy 625 specimen. The TEM observations showed that a high density of tangled dislocations and irradiation-induced defect clusters formed in the stainless steels and Ni-based alloys irradiated at 485 degrees C. At 668 degrees C, the material microstructures coarsened and their dislocation density decreased significantly. Long rod-like precipitates of Zr(Cr, Fe) compounds formed in the H1 and H2 steels that were modified with Zr. The yield stress drop of T3 steel in tensile stress was observed and is caused by grain-size coarsening at an irradiation of 668 degrees C.

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