Journal
CHEMELECTROCHEM
Volume 6, Issue 13, Pages 3355-3366Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/celc.201900743
Keywords
metal-organic framework; CC@CoMoO4-Co(OH)(2) nanosheets; asymmetric supercapacitors; binder-free flexible devices
Categories
Funding
- National Natural Science Foundation of China [51603053, 51872057, 51672054, 21576060]
- National Natural Science Foundation of Heilongjiang Province [E2016019]
- Fundamental Research Funds of the Central University [3072019CF1003]
- China Postdoctoral Science Foundation [2019M651260]
- Defense Industrial Technology Development Program [JCKY2016604C006]
- National Key Research and Development Program of China [2016YFE0202700]
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Due to the urgent demand for portable electronics, enormous research efforts are devoted for the development of flexible, wearable and lightweight supercapacitors. Herein, we report a cost-effective chemical liquid process followed with a refluxing route to grow CC@CoMoO4-Co(OH)(2) nanosheets with Co-based MOF as precursor. The resulting CC@CoMoO4-Co(OH)(2)-4 electrode delivers a significantly enhanced specific capacitance of 2028 F g(-)1 at 1 A g(-1) and capacitance of 1581.8 F g(-1) at 20 A g(-1). Furthermore, the flexible all-solid-state asymmetric supercapacitor (CC@CoMoO4-Co(OH)(2)//AC) is assembled, displays a high energy density of 61 Wh kg(-1) at power density of 800 W kg(-1), with an excellent cycle stability. These exceptional electrochemical performances could be ascribed to the unique structure and multi-metal ion combination contributes to the ideal synergistic effects, which also signify that the potential application of CC@CoMoO4-Co(OH)(2) nansheets in high-performance supercapacitors.
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