Journal
TETRAHEDRON
Volume 75, Issue 41, Pages -Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tet.2019.130490
Keywords
Cyclopropanol; Ring opening reaction; Silver catalysis; Chroman-4-ones; Indanones
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Funding
- Science Foundation for Distinguished Scholars of Dongguan University of Technology [GC200906-10]
- Postdoctor Foundation of Dongguan University of Technology [196100040006]
- leading talents of innovation and entrepreneurship of the Dongguan City [D2017 (16)]
- National Natural Science Foundation of China [51773165]
- Young Talent Support Plan of Xi'an Jiaotong University
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A variety of chroman-4-one and indanone derivatives were conveniently synthesized from readily available cyclopropanols and alkenyl aldehydes via a silver catalyzed radical ring-opening/coupling/cyclization cascade. The reaction proceeded under mild and neutral conditions with broad substrate scope and afforded the desired products in moderate to good yields. A probable mechanism for the cascade reaction was also proposed. (C) 2019 Published by Elsevier Ltd.
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