Journal
SENSORS AND ACTUATORS B-CHEMICAL
Volume 288, Issue -, Pages 232-242Publisher
ELSEVIER SCIENCE SA
DOI: 10.1016/j.snb.2019.02.093
Keywords
S, N: graphene quantum dots; Polyaniline; Metal-organic framework; In-situ polymerization; Acetone sensor
Funding
- National Natural Science Foundation of China [51777215]
- Key Research & Development Plan Project of Shandong Province [2018GSF117002]
- Fundamental Research Funds for the Central Universities of China [18CX07010A]
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Metal-organic frameworks-derived zinc oxide nanopolyhedra/S, N: graphene quantum dots/polyaniline (ZnO/S, N: GQDs/PANI) ternary nanohybrid was synthesized by in-situ polymerization route. The ZnO/S, N: GQDs/PANI nanocomposite was fabricated on a flexible polyethylene terephthalate (PET) substrate with interdigital electrodes. The acetone-sensing properties of the ZnO/S, N: GQDs/PANI nanocomposite sensor were investigated by exposing it to various concentrations of acetone at room temperature. The ZnO/S, N: GQDs/PANI sensor demonstrated high response, fast response/recovery time, stable repeatability, excellent selectivity, outstanding long-term stability, and ppb-level sensitivity for trace acetone detection at room temperature. These results render the ZnO/S, N: GQDs/PANI film sensor a promising candidate for acetone sensing at room temperature. The underlying sensing mechanism of the ZnO/S, N: GQDs/PANI sensor toward acetone gas ascribed to the synergistic effect and heterojunction created in the ZnO/S, N: GQDs/PANI nanocomposite.
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