Journal
SCIENCE OF THE TOTAL ENVIRONMENT
Volume 668, Issue -, Pages 1165-1174Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.scitotenv.2019.03.095
Keywords
GO/PAA hydrogel; Cd-2(+) adsorption; Adsorbent recycle; Photocatalyst
Categories
Funding
- Taishan Scholar Foundation of Shandong Province [ts201511003]
- Key Research Projects of Shandong Province [2017GSF17109]
- Major Technological Innovation Engineering Project of Shandong Province [2018CXGC1010]
- National Natural Science Foundation of China [21677088]
- Young Scholars Program of Shandong University [2015WLJH34]
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In this work, a GO (graphene oxide)/PAA (poly acrylic acid) hydrogel was prepared by graft polymerization between GO and AA. It was employed as highly efficient adsorbent for Cd2+ removal from wastewater. The GO/PAA-Cd2+ composite after the adsorption process was recycled through in-situ precipitation to obtain GO/PAA-Cd2+ composites. During the synthesis process, the amounts of GO and M were optimized to enable the hydrogel with maximum adsorption of Cd2+ (316.4 mg/g at 25 degrees C). The structure and chemical composites of GO/PAA hydrogel were investigated through FTIR spectra, Raman spectra, and TGA. The adsorption kinetics and isotherms of Cd2+ on GO/PAA were analyzed. The synthesized products served as an efficient adsorbent for Cd2+ and a suitable matrix for the CdS quantum dots formation which was confirmed by various characterizations, including XPS, SEM-EDS and HRTEM. The roles of GO and PM in the successive adsorption-photocatalyst process were proved to be complementary: PAA improved the adsorption of Cd2+ while GO enhanced the photocatalyst efficiency. The photodegradation rate of MB (30 mg/L) was over 90% within 2 h. (C) 2019 Elsevier B.V. All rights reserved.
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