4.7 Article

Fabrication of conductive and high-dispersed Ppy@Ag/g-C3N4 composite photocatalysts for removing various pollutants in water

Journal

APPLIED SURFACE SCIENCE
Volume 387, Issue -, Pages 366-374

Publisher

ELSEVIER SCIENCE BV
DOI: 10.1016/j.apsusc.2016.06.124

Keywords

Ppy@Ag/g-C3N4 photocatalyst; Various pollutant remove; Effective charge separation; Visible light irradiation; Mediator

Funding

  1. National Natural Science Foundation of China [21546013, U1510126]
  2. University Professional Degree Postgraduate Research Practice Program of Jiangsu Province [SJZZ_0136]
  3. Innovation Program Foundation of Jiangsu Province [SKYLX15_1089]

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The ternary conductive Ppy@Ag/g-C3N4 composite photocatalysts was successfully synthesized by polymerization process and surface polymerization technique. And the as-prepared Ppy@Ag/g-C3N4 sample exhibited the higher photocatalytic activity for various pollutant (MO, DM, TC, CIP, GFLX and EH) remove than that of pure g-C3N4 and Ag/g-C3N4 under visible light irradiation. It mainly originated from the Ag nanoparticles anchored between g-C3N4 and Ppy acted as electron transfer mediator that facilitated the charge carrier separation and then expending the lifetime of the carriers. Meanwhile, the obtained Ppy@Ag/g-C3N4 sample also showed a relatively good recycling stability which was the crucial factor for photocatalyst practical application. This work provided a new facile strategy for improving photo-degradation activity of g-C3N4 photocatalyst. (C) 2016 Elsevier B.V. All rights reserved.

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