Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 141, Issue 30, Pages 11801-11805Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.9b05571
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Funding
- Spanish MINECO [CTQ2017-84692-R]
- EU Feder Funding, South Korea ADD's research project [912412201]
- Polish NCN Miniatura 1 grant [2017/01/X/ST5/00101]
- Comunidad de Madrid TALENTO grant [2017-T1/IND5148]
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UiO-66, MOF-808 and NU-1000 metal-organic frameworks exhibit a differentiated reactivity toward [Mg(OMe)(2)(MeOH)(2)](4) related to their pore accessibility. Microporous UiO-66 remains unchanged while mesoporous MOF-808 and hierarchical micro/mesoporous NU-1000 materials yield doped systems containing exposed MgZr5O2(OH)(6) clusters in the mesoporous cavities. This modification is responsible for a remarkable enhancement of the catalytic activity toward the hydrolytic degradation of P-F and P-S bonds of toxic nerve agents, at room temperature, in unbuffered aqueous solutions.
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