Journal
JOURNAL OF POWER SOURCES
Volume 424, Issue -, Pages 158-164Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.jpowsour.2019.03.103
Keywords
V2O5; Hierarchical structure; Lithium ion battery; Sustainable; Recycling process; LiV2O5
Funding
- National Natural Science Foundation of China [51872139, 21501091]
- NSF of Jiangsu Province [BK20170045, BK20150064]
- Recruitment Program of Global Experts [1211019]
- Six Talent Peak Project of Jiangsu Province [XCL-043]
- National Key Basic Research Program of China (973) [2015CB932200]
- China Postdoctoral Science Foundation [2016M600404, 2017T100360]
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A versatile synthetic approach is demonstrated to fabricate vanadium pentoxide hierarchical structures with three-dimensional electron carriers as anode materials for lithium-ion battery. Such unique structures are favorable for providing easy access of electrolyte to the electrode during lithiation-delithiation process and also shortening the pathway of the ion and electron transport, which guarantee excellent electrochemical performance. As a consequence, high specific capacities of 960 mAh g(-1) at 200 mA g(-1) and 738 mAh g(-1) at 500 mA g(-1) after 300 cycles are achieved without obvious decay. More remarkably, it is essential to rebuild a new recycling process owing to the massive waste produced by dealing with spent lithium-ion battery. Therefore, an energy-saving and environment-friendly process is introduced to recycle the used V2O5 batteries. Through a facile annealing process, LiV3O8 is obtained and reused as sustainable anode materials for the first time. The recycled product LiV3O8 delivers excellent electrochemical performance, e.g., a high capacity of 542 mAh g(-1) at 200 rnA g(-1) and the coulombic efficiency of over 99% after 600 cycles. This finding not only promotes the development of vanadium oxides for lithium-ion battery, but also sheds light on searching potential protocol for metal ion battery recycling.
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