Journal
FUNCTIONAL MATERIALS LETTERS
Volume 12, Issue 6, Pages -Publisher
WORLD SCIENTIFIC PUBL CO PTE LTD
DOI: 10.1142/S1793604719500796
Keywords
alpha-Fe2O3; protoporphyrin IX; photocatalysis; electron transfer; organic-inorganic hybrid composites
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Funding
- National Natural Science Foundation of China [51302019, 21703014]
- Science and Technology Development Project Foundation of Jilin Province [20180520222JH]
- Industrial Technology Research Project [2018C043-3]
- Jilin Provincial Science Education 13th Five-Year Project [GH16104]
- Scientific and Technological 13th Five-Year Plan Project of Jilin Provincial Department of Education [JJKH20191195KJ]
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As a novel strategy for improving the photocatalytic activity through hybrid with small molecule photosensitizer, alpha-Fe2O3 has been successfully functionalized with protoporphyrin IX (PPIX) in order to enhance sunlight-driven photocatalytic degradation of dyes and antimicrobial activity due to the staggered energy band structures which promote a charge transfer between alpha-Fe2O3 and PPIX and generate free holes and electrons. The results show that alpha-Fe2O3 could absorb more sunlight and generate more free electrons and holes after being decorated with PPIX. As a result, PPIX-functionalized alpha-Fe2O3 has an enhanced photocatalytic degradation of dyes ability against rhodamine B and methyl orange and antimicrobial activity against Escherichia coli. The present strategy gives a promising way to prepare photocatalytic agent hybrid with small molecule photosensitizer.
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