Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 58, Issue 32, Pages 10985-10989Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201905445
Keywords
dual-control; macroscopic actuation; molecular motor; soft materials; supramolecular polymer
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Funding
- Croucher Foundation (Croucher Postdoctoral Fellowship)
- Netherlands Organization for Scientific Research (NWOCW)
- European Research Council (ERC) [694345]
- Ministry of Education, Culture and Science [024.001.035]
- Ministry of Education, Culture, Sports, Science and Technology (MEXT), Japan [26102008, 15K21721]
- Grants-in-Aid for Scientific Research [15K21721] Funding Source: KAKEN
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Three-dimensional unidirectionally aligned and responsive supramolecular hierarchical assemblies have much potential in adaptive materials for biomedical and soft actuator applications. However, to achieve systematical control of the motion of stimuli-responsive materials by orthogonal external stimuli and to complete a series of complicated tasks remains a grand challenge. Herein, we demonstrate a novel designed hybrid supramolecular assembly of molecular motor amphiphiles that also serves as a template for iron nanoparticles growth, and as a consequence this soft hybrid material is orthogonally controlled by dual light/magnetic stimuli. Macroscopic motor amphiphile strings, decorated with iron nanoparticles, provide fast response photoactuations and magnet induced movements that allows a precisely controlled cargo transport process.
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