Journal
ADVANCED SYNTHESIS & CATALYSIS
Volume 361, Issue 18, Pages 4237-4242Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.201900712
Keywords
Photocatalysis; visible light; alkylarylation; nitrogenous heterocycles; C-H functionalization
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Funding
- National Natural Science Foundation of China [21502086, 41575118]
- Natural Science Foundation of Fujian Province [2019J01744]
- Outstanding Youth Science Foundation of Fujian Province [2015J06009]
- Program for Excellent Talents of Fujian Province
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Radical cascade oxidative alkylarylations of N-aryl/benzoyl acrylamides have been established through visible-light-enabled photocatalysis, furnishing a wide variety of functionalized oxindoles and isoquinolinediones in good-to-excellent yields under the synergistic interactions of an organic fluorophores-type photocatalyst 4CzIPN, trifluoroacetoxyiodobenzene (PIFA), and 1,3,5-trimethoxybenzene with visible light irradiation. The prominent features of this method are the broad substrate scope, excellent functional group tolerance, and mild reaction conditions.
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