4.8 Article

High-Performance Transparent Quantum Dot Light-Emitting Diode with Patchable Transparent Electrodes

Journal

ACS APPLIED MATERIALS & INTERFACES
Volume 11, Issue 29, Pages 26333-26338

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsami.9b05969

Keywords

silver nanowire; patchable; transparent; thermal release tape; quantum dot light-emitting diode

Funding

  1. National Research Foundation (NRF) of Korea - Ministry of Science, Information and Communications Technology [NRF-2018R1C1B5043900, 2019K1A3A1A25000230]
  2. National Research Foundation of Korea [2019K1A3A1A25000230] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)

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Patchable electrodes are attractive for applications in optoelectronic devices because of their easy and reliable processability. However, development of reliable patchable transparent electrodes (TEs) with high optoelectronic performance is challenging; till now, optoelectronic devices fabricated with patchable TEs have been exhibiting limited performance. In this study, Ag nanowire (AgNW)/poly(methyl methacrylate) (PMMA) patchable TEs are developed and the highly efficient transparent quantum dot light-emitting diodes (QLEDs) using the patchable TEs are fabricated. AgNWs with optimized optoelectronic properties (figure of merit 3.3 X 10(-2)) are coated by an ultrathin PMMA nanolayer and transferred to thermal release tapes that enable physical attachment of TEs on the QLEDs without a significant damage to the adjacent active layer. The transparent QLEDs using patchable transparent top electrodes display excellent performance, with the maximum total luminance and current efficiency of 27 310 cd.m(-2) and 45.99 cd.A(-1), respectively. Fabricated by all-solution-based processes, these QLEDs exhibit the best performance to date among devices adopting patchable top electrodes.

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