4.8 Article

Emergent Topological Hall Effect in La0.7Sr0.3MnO3/SrIrO3 Heterostructures

Journal

ACS APPLIED MATERIALS & INTERFACES
Volume 11, Issue 23, Pages 21268-21274

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsami.9b05562

Keywords

topological Hall effect; noncoplanar spin texture; interface coupling; Dzyaloshinskii-Moriya interactions; SrIrO3

Funding

  1. State Key Program for Basic Research of China [2015CB921203]
  2. Natural Science Foundation of China [51725203, 51721001, 51702153, 51402149]
  3. Natural Science Foundation of Jiangsu Province [BK20160627]
  4. Max Planck POSTECH/KOREA Research Initiative Program through National Foundation of Korea - Ministry of Science, ICT, and Future Planning [2016K1A4A4A01922028]
  5. National Research Foundation of Korea [2016K1A4A4A01922136] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)

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Recently, perovskite oxide heterostructures have drawn great attention because multiple and complex coupling at the heterointerface may produce novel magnetic and electric phenomena that are not expected in homogeneous materials either in the bulk or in films. In this work, we report for the first time that an emergent giant topological Hall effect (THE), associated with a noncoplanar (NC) spin texture, can be induced in ferromagnetic (FM) La(0.7)Sr(0.3)MnO(3)thin films in a wide temperature range of up to 200 K by constructing La0.7Sr0.3MnO3/SrIrO3 epitaxial heterostructures on (001) SrTiO3 substrates. This THE is not observed in La0.7Sr0.3MnO3 single-layer films or La0.7Sr0.3MnO3/SrlrO(3)/SrIrO3 trilayer heterostructures, indicating the relevance of the La0.7Sr0.3MnO3/SrlrO(3) interface, where the Dzyaloshinskii-Moriya interaction due to strong spin-orbital coupling in SrIrO3 may play a crucial role. The fictitious field associated with THE is independent of temperature in La0.7Sr0.3MnO3/SrIrO3 heterostructures, suggesting that the NC spin texture may be magnetic skyrmions. This work demonstrates the feasibility of using SrIrO3 to generate novel magnetic and transport characteristics by interfacing with other correlated oxides, which might be useful to novel spintronic applications.

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