4.8 Article

Fluorescent Fluid in 3D-Printed Microreactors for the Acceleration of Photocatalytic Reactions

Journal

ADVANCED SCIENCE
Volume 6, Issue 13, Pages -

Publisher

WILEY
DOI: 10.1002/advs.201900583

Keywords

3D printing; fluorescent fluids; light-converting media; microreactors; photochemistry

Funding

  1. National Natural Science Foundation of China [51703017, 21872018]
  2. China Postdoctoral Science Foundation [2016M601302]
  3. Fundamental Research Funds for the Central Universities [DUT17LK36, DUT18RC(4)013]

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The photochemical microreactor has been a burgeoning field with important application in promoting photocatalytic reactions. The integration of light-converting media and microflow chemistry renders new opportunity for efficient utilization of light and high conversion rate. However, the flexibility of emission light wavelength regulation and the universality of the microreactor remain significant problems to be solved. Here, a photochemical microreactor filled with fluorescent fluid is fabricated by a 3D printing technique. The light-converting medium in the fluorescent fluid is used to collect and convert light, and then delivers light energy to the embedded continuous-flow reaction channels to promote the chemical reaction process. With the merits of flowability, different light-converting media can be replaced, making it a general tool for photocatalytic reactions in rapid screening, parameters optimization, and kinetic mechanism research.

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