Journal
ENERGY TECHNOLOGY
Volume 7, Issue 6, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ente.201900271
Keywords
biomass; heterogeneous catalysis; mesoporous materials; synergetic effect; zeolites
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Funding
- National Natural Science Foundation of China [21722103, 21720102002, 21673140]
- Shanghai Basic Research Program [16JC1401600]
- SJTU-MPI partner group
- Shanghai Rising-Star Program [16QA1402100]
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In this article, the synergetic effect between the B- and Al-based acidic sites in B-Al co-doped mesoporous MFI nanocrystals (denoted as m-B-Al-S1) is rationally applied to modify the alcoholysis process of furfuryl alcohol. The porosity and dopant concentration of the m-B-Al-S1 materials are optimized via a modified Kirkendall growth method to boost the ultra-high selectivity to ethyl levulinate reactions (94%). The m-B-Al-S1 catalyst also shows good stability for further reuses.
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