Journal
ADVANCED MATERIALS INTERFACES
Volume 6, Issue 13, Pages -Publisher
WILEY
DOI: 10.1002/admi.201900359
Keywords
aerosol deposition; CsPbBr3; Al2O3 nanocomposite; photoluminescence; thermal stability
Funding
- National Research Foundation of Korea (NRF) [2014R1A5A1009799, 2017R1C1B5017013]
- Nano-Material Technology Development Program, Republic of Korea [2017M3A7B4041696]
- National Research Foundation of Korea [2017R1C1B5017013, 2017M3A7B4041696] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
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Luminescent perovskite structure has been used in a polymer-encapsulated form for display applications. However, insulating polymers as a host matrix are intrinsically vulnerable to thermal stresses which cause softening distortion or deterioration in thermoplastic polymers. Here, nanostructured CsPbBr3/Al2O3 composite film is developed by aerosol deposition method. At first, CsPbBr3/Al2O3 composite powders with bright and saturated green emission are synthesized. Then, the ceramic composite powder comprising monoclinic CsPbBr3 nanocrystals supported on submicron alpha-Al2O3 particles is successfully transformed to a film-type by aerosol deposition, which enables a nonsolvent-induced process at room temperature. The deposited films show a pure green spectrum with a narrow full width at half maximum of 17 nm, high long-term stability at 150 degrees C for over 20 d, and an absolute photoluminescence quantum yield of 8%-15%. In general, inorganic films are known to have difficulty with flexibility and patterns. However, the deposited film can be employed in useful applications such as down-converting materials for an LCD backlight with a wide-color gamut of 89.2% in Rec. 2020, highly flexible ceramic composite films, multilayer films, patterning of surfaces for an advanced color filter array, and deposition on curved substrates toward diverse display fields.
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