Journal
SCIENCE OF THE TOTAL ENVIRONMENT
Volume 663, Issue -, Pages 68-77Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.scitotenv.2019.01.326
Keywords
Black odorous river; Sediment internal loading; Remediation; Nutrient release; Mobile phosphorus
Categories
Funding
- State Major Project of Water Pollution Control and Management [2017ZX07603-005]
- National Natural Science Foundation of China [51579233]
- Key Development Program of Jiangsu Province [BE2016811]
- 135 project of NIGLAS [NIGLAS2018GH05]
- Opening Fund of the State Key Laboratory of Environmental Geochemistry [SKLEG2018909]
- Nanjing Social Development Project [201716001]
- CAS Interdisciplinary Innovation Team [JCTD-2018-16]
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The continuous release of nutrients from sediment is a major barrier to the remediation of black odorous rivers. This study used a long-term laboratory incubation experiment to investigate the effectiveness of sediment dredging, intermittent aeration, and in situ inactivation with modified clays to reduce the internal loading of sediment from a seriously polluted river. The results indicated that intermittent aeration and in situ inactivation were effective in reducing the TN and NH4+ concentrations in the water column. However, sediment dredging did not consistently reduce the TN and NH4+ concentrations in the water column. In contrast, the three methods were all effective in controlling the TP and PO43- concentrations in the water column. Except for dredging, >30% of NH4+ and 40% of PO43- fluxes from sediment were reduced when compared with a control sample after 120 days of remediation. Dredging induced a significant release of NH4+ from sediment. Dredging and aeration made nearly no change to the amount of extractable nitrogen in the sediment. However, inactivation may increase sediment-extractable ammonium in deep sediment layers with time due to vertical transportation of clay by intensive bio-turbation. Dredging is the most effective way to reduce surface mobile phosphorus over time while the transported clays can reduce a large percentage of the mobile phosphorus in deeper sediment. The relative abundance of Nitrospira in the surface sediment increased significantly with each remediation measure, creating favorable conditions for the reduction of the ammonium released from sediment. Altogether, the results of this study indicated that clay inactivation is the best method for controlling the internal loading of both phosphorus and nitrogen in seriously polluted river sediment. (C) 2019 Elsevier B.V. All rights reserved.
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