Journal
ORGANIC LETTERS
Volume 21, Issue 11, Pages 3959-3962Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.9b01101
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Funding
- National Natural Science Foundation of China [NSFC21572272]
- Foundation of The Open Project of State Key Laboratory of Natural Medicines [SKLNMZZCX201818]
- Fundamental Research Funds for the Central Universities [2632018ZD02]
- Innovation Team of the Double-First Class Disciplines [CPU2018GY04, CPU2018GY35]
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A Rh(III)-catalyzed intramolecular olefin hydroarylation of aromatic aldehydes with a transient directing group has been described. The bidentate directing groups in situ generated from aromatic aldehydes and beta-alanine could enable the subsequent C-H activation and hydroarylation with excellent site selectivities and high functional group compatibility. The further conversion of the aldehyde group showcased the broad application prospects of this methodology.
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