4.7 Article

One-Pot, Three-Component Approach to Diarylmethylphosphonates: A Direct Entry to Polycyclic Aromatic Systems

Journal

JOURNAL OF ORGANIC CHEMISTRY
Volume 84, Issue 10, Pages 6323-6336

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.9b00668

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Funding

  1. National Research Foundation of Korea [NRF-2017R1A2A2A05069364, NRF-2018R1A6A1A03023718]

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A new type of three-component reaction was developed consisting of aldehydes, electron-rich (hetero)arenes, and trialkyl phosphite, which provided facile access to a wide range of diarylmethylphosphonates under mild reaction conditions. Simple one- or two-step synthetic manipulation of the resulting compounds enabled us to reach several polycyclic (hetero)aromatic systems efficiently.

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