Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 84, Issue 10, Pages 6475-6482Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.9b00525
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Funding
- Natural Science Basic Research Plan in Shaanxi Province of China [2016JZ002]
- National Natural Science Foundation of China [21602168]
- Key Laboratory Construction Program of Xi'an Municipal Bureau of Science and Technology [201805056ZD7CG40]
- Fundamental Research Funds of the Central Universities [zrzd2017001, xjj2016056]
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An efficient iminyl radical-triggered 1,5-hydrogen-atom transfer/Heck-type coupling cascade has been achieved through visible-light photoredox catalysis. A variety of unactivated C(sp(3))-H bonds have been alkenylated efficiently and selectively with easily available alkenes, providing an elegant route to gamma-alkenylated ketone.
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