Journal
CORROSION SCIENCE
Volume 156, Issue -, Pages 58-70Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.corsci.2019.05.006
Keywords
CO2 corrosion; High temperature; Iron carbonate; Calcium carbonate; Mixed carbonate
Funding
- EPSRC [1812412] Funding Source: UKRI
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The role of Ca2+ ions on the corrosion behaviour of carbon steel in CO2-corrosion environments was evaluated at 80 degrees C and 150 degrees C. In the presence of Ca2+ ions there was a more significant effect on the general corrosion rate at the lower temperature of 80 degrees C where the protection afforded by the corrosion product layer was reduced. The extent of localised/pitting corrosion increased through the addition of Ca2+ ions indicating that Ca2+ plays a role in promoting localised corrosion. XRD based calculations, along with focused ion beam EDX-line scans confirmed that the mixed Ca/Fe carbonates precipitated with concentration gradients across their thicknesses.
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