Journal
CHEMCATCHEM
Volume 11, Issue 15, Pages 3355-3365Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cctc.201900770
Keywords
on-the-fly catalyst modification; structure-performance relationship; hydrogenation; flow catalysis; laboratory X-ray photon-in photon out spectroscopy
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Hydrogenation is a quintessential process to the chemical industry. It is heavily involved in organic synthesis and fuel production, among other processes. Preferentially the reactions are carried out with heterogeneous catalysts and when possible in flow mode. Herein, we provide a retrospective on selective surface modification of catalysts for improved selectivity and understanding of catalytic reactivity. In addition, we provide a prospectus for an emerging strategy of carrying out surface modification on-the-fly to produce novel catalysts in a fast and reproducible way and to understand catalytic phenomena.
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