Journal
ADVANCED MATERIALS
Volume 31, Issue 31, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.201808066
Keywords
electrocatalysis; electrolyzers; fuel cells; hydrogen evolution; hydrogen oxidation
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Funding
- National Science Foundation of China [21773171]
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Electrochemical energy storage and conversion through hydrogen is essential for a clean and sustainable energy system. Highly efficient hydrogen electrocatalysts play a key role in the electrochemical transformation reactions. A comprehensive understanding of the hydrogen reaction kinetics and mechanisms is critical for the catalyst design and development. Especially pH-dependent hydrogen evolution and oxidation reaction (HER/HOR) kinetics receives increasing interest, and understanding its origin adds new knowledge to fundamental hydrogen electrocatalysis. Here, a detailed description of kinetic analysis and reaction mechanisms for HER/HOR, and a brief summary about recent development of highly efficient and cost-effective hydrogen electrocatalysts are presented. Lastly, recent advances in the fundamental understanding of pH-dependent hydrogen electrocatalysis are discussed.
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