Journal
ADVANCED MATERIALS
Volume 31, Issue 25, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.201808205
Keywords
artificial photosynthesis; mixed anion compounds; solar energy conversion; solar fuel; water oxidation
Categories
Funding
- [JP16H06130]
- [JP16H06441]
- [JP17K19169]
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CO2 reduction to carbon feedstocks using heterogeneous photocatalysts is an attractive means of addressing both climate change and the depletion of fossil fuels. Of particular importance is the development of a photosystem capable of functioning in response to visible light, which accounts for the majority of the solar spectrum, representing a kind of artificial photosynthesis. Hybrid systems comprising a metal complex and a semiconductor are promising because of the excellent electrochemical (and/or photocatalytic) activity of metal complexes during CO2 reduction and the ability of semiconductors to efficiently oxidize water to molecular O-2. Here, the development of hybrid photocatalysts and photoelectrodes for CO2 reduction in combination with water oxidation is described.
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