Journal
ASIAN JOURNAL OF ORGANIC CHEMISTRY
Volume 8, Issue 5, Pages 722-730Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ajoc.201900018
Keywords
pyrene; fluorine atom; Intramolecular charge transfer; n-type semiconductor
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Funding
- National Natural Science Foundation of China [21511130059]
- Royal Society of United Kingdom of Great Britain [21511130059]
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Mono- and 1,6-disubstituted pyrene derivatives bearing perfluorotoluene or perfluorobenzonitrile moieties were synthesized by nucleophilic substitution processes. The compounds were characterized by NMR, UV-vis, photoluminescence (PL), thermal gravimetric analysis (TGA), differential scanning calorimetry (DSC), cyclic voltametry (CV) and density functional theory (DFT) calculations. It was found that derivatives substituted with perfluorobenzonitrile showed better thermal stability, stronger electron withdrawing ability and better fluorescence properties than the corresponding perfluorotoluyl-pyrene systems
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