Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 56, Issue 2, Pages 559-562Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201610182
Keywords
dehydrogenation; homogeneous catalysis; ligand design; manganese; methanol
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Funding
- VCI [196241]
- EU fund H2020-MSCA-ITN in Horizon 2020 as part of the NoNoMeCat
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For the first time, structurally defined manganese pincer complexes catalyze the dehydrogenation of aqueous methanol to hydrogen and carbon dioxide, which is a transformation of interest with regard to the implementation of a hydrogen and methanol economy. Excellent long-term stability was demonstrated for the Mn-PNPiPr catalyst, as a turnover of more than 20000 was reached. In addition to methanol, other important hydrogen carriers were also successfully dehydrogenated.
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