Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 55, Issue 32, Pages 9178-9182Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201602429
Keywords
mesoporous materials; nanocrystals; palladium; shape-selective catalysis; zeolites
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Funding
- National Basic Research Program of China [2013CB934102]
- National Natural Science Foundation of China [21331004, 21301116]
- Shanghai Eastern Scholar Program
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Pd nanoparticles were successfully encapsulated inside mesoporous silicalite-1 nanocrystals (Pd@mnc-S1) by a one-pot method. The as-synthesized Pd@mnc-S1 with excellent stability functioned as an active and reusable heterogeneous catalyst. The unique porosity and nanostructure of silicalite-1 crystals endowed the Pd@mnc-S1 material general shape-selectivity for various catalytic reactions, including selective hydrogenation, oxidation, and carbon-carbon coupling reactions.
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