4.8 Article

High-Performance Lithium-Air Battery with a Coaxial-Fiber Architecture

Journal

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 55, Issue 14, Pages 4487-4491

Publisher

WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201511832

Keywords

carbon nanotube; flexible devices; gel electrolyte; lithium-air battery; wearable devices

Funding

  1. NSFC [21225417, 51573027, 51403038]
  2. STCSM [15XD1500400, 12nm0503200, 15JC1490200]
  3. Program for Outstanding Young Scholars from Organization Department of the CPC Central Committee

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The lithium-air battery has been proposed as the next-generation energy-storage device with a much higher energy density compared with the conventional lithium-ion battery. However, lithium-air batteries currently suffer enormous problems including parasitic reactions, low recyclability in air, degradation, and leakage of liquid electrolyte. Besides, they are designed into a rigid bulk structure that cannot meet the flexible requirement in the modern electronics. Herein, for the first time, a new family of fiber-shaped lithium-air batteries with high electrochemical performances and flexibility has been developed. The battery exhibited a discharge capacity of 12470mAhg(-1) and could stably work for 100cycles in air; its electrochemical performances were well maintained under bending and after bending. It was also wearable and formed flexible power textiles for various electronic devices.

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