Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 55, Issue 32, Pages 9321-9325Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201603211
Keywords
carbon dioxide; gas separation; membranes; montmorillonite
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Funding
- Natural Science Foundation of China [20836006, 21436009]
- National High-tech Research and Development Project [2012AA03A611]
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Highly permeable montmorillonite layers bonded and aligned with the chain stretching orientation of polyvinylamineacid are immobilized onto a porous polysulfone substrate to fabricate aligned montmorillonite/polysulfone mixed-matrix membranes for CO2 separation. High-speed gas-transport channels are formed by the aligned interlayer gaps of the modified montmorillonite, through which CO2 transport primarily occurs. High CO2 permeance of about 800 GPU is achieved combined with a high mixed-gas selectivity for CO2 that is stable over a period of 600 h and independent of the water content in the feed.
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