Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 55, Issue 35, Pages 10336-10339Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201605266
Keywords
aerosols; alkenes; atmospheric chemistry; organosulfates; sulfur dioxide
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Funding
- Agence Nationale de la Recherche through COGNAC grant [ANR-13-BS06-0002-01]
- Marie Curie International Research Staff Exchange project AMIS Grant [295132]
- European Research Council under European Union/ERC [290852-AIRSEA]
- Agence Nationale de la Recherche (ANR) [ANR-13-BS06-0002] Funding Source: Agence Nationale de la Recherche (ANR)
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The heterogeneous reaction between SO2 and unsaturated compounds results in the efficient production of organosulfates for several fatty acids and long-chain alkenes. The presence of an acid group, the physical state of the reactants (solid or liquid), the nature of the double bond (cis, trans, terminal), and the use of light irradiation all have an impact on the reaction rate. The reaction was investigated using different set-ups (coated flow tube, aerosol flow tube, and diffuse reflectance infrared Fourier transform cell). The reaction products were identified by high-resolution mass spectrometry and the impact of this reaction on organosulfate formation in the atmosphere is discussed.
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