Journal
ORGANIC LETTERS
Volume 21, Issue 9, Pages 2973-2977Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.9b00307
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Funding
- National Natural Sciences Foundation of China [21871044, 21472017]
- Natural Sciences Foundation of Jilin Province [20190201073JC]
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A rhodium-catalyzed coupling-cyclization reaction of alkenyldiazoacetates with o-alkenyl arylisocyanides has been developed. In this reaction, the highly reactive alkenylketenimine intermediates generated by coupling reaction of alkenyldiazoacetates with o-alkenyl arylisocyanides undergo intramolecular [4 + 2] cycloaddition and provide a novel, highly efficient method for the one-step synthesis of carbazoles by formation of three new bonds and two rings from readily available acyclic starting materials.
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