Journal
ORGANIC LETTERS
Volume 21, Issue 6, Pages 1857-1862Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.9b00444
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Funding
- National Natural Science Foundation of China [21472082, 21402088, 21772085]
- Fundamental Research Funds for the Central Universities [020514380148]
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Difunctionalization of olefins represents a powerful synthetic tool and yet a challenging task. This work describes an electrochemically enabled fluoroalkylation migration reaction of unactivated olefins in the absence of a strong oxidant or heavy metal catalyst, affording fluorinated (hetero)aryl ketones in good yields and excellent regioselectivities. The efficient and sustainable electrochemical strategy provides a rapid access to a dual functionalized fluorine-containing heterocyclic manifold.
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