Journal
ORGANIC LETTERS
Volume 21, Issue 4, Pages 1116-1120Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.9b00034
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Funding
- Austrian Science Fund (FWF) [P29584-N28]
- Austrian Science Fund (FWF) [P29584] Funding Source: Austrian Science Fund (FWF)
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An efficient synthesis of quinolines, pyrimidines, quinoxalines, pyrroles, and aminomethylated aromatic compounds catalyzed by a well-defined Re(I) PNP pincer complex is described. All reactions proceed with liberation of dihydrogen and elimination of water. Under optimized reaction conditions a wide range of organic functional groups are tolerated. This study demonstrates that rhenium catalysts are performing extremely well in dehydrogenative processes with considerably lower catalyst loadings and shorter reaction times when compared to analogous Mn(I) complexes.
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