Journal
ORGANIC LETTERS
Volume 21, Issue 4, Pages 917-920Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.8b03865
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Funding
- Natural Science Basic Research Plan in Shaanxi Province of China [2016JZ002]
- National Natural Science Foundation of China [21602168]
- Key Laboratory Construction Program of Xi'an Municipal Bureau of Science and Technology [201805056ZD7CG40]
- Fundamental Research Funds of the Central Universities [zrzd2017001, xjj2016056]
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An efficient iron-catalyzed intermolecular remote C(sp(3))-H heteroarylation of alkyl ketones has been developed via an iminyl radical-triggered 1,5-hydrogen-atom transfer (HAT) cascade. This protocol was amenable to a wide variety of alkyl ketones and heteroaryls, thus providing a straightforward method for the late-stage functionalization of alkylketones and heteroaryls.
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