4.8 Article

Determining Interaction Enhanced Valley Susceptibility in Spin-Valley-Locked MoS2

Journal

NANO LETTERS
Volume 19, Issue 3, Pages 1736-1742

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.8b04731

Keywords

Transition metal dichalcogenide; quantum oscillation; Landau level; Zeeman effect; g-factor; electron-electron interaction

Funding

  1. Research Grants Council of Hong Kong [16300717, SBI17SC16]
  2. FB417-UoM-HKUST
  3. Hong Kong Ph.D. Fellowship
  4. Army Research Office [W911NF-18-1-0416]
  5. graphene flagship project [604391]
  6. LNCMI-CNRS

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Two-dimensional transition metal dichalcogenides (TMDCs) are recently emerged electronic systems with various novel properties, such as spin-valley locking, circular dichroism, valley Hall effect, and superconductivity. The reduced dimensionality and large effective masses further produce unconventional many-body interaction effects. Here we reveal strong interaction effects in the conduction band of MoS2 by transport experiment. We study the massive Dirac electron Landau levels (LL) in high-quality MoS2 samples with field-effect mobilities of 24 000 cm(2)/(V.s) at 1.2 K. We identify the valley-resolved LLs and low-lying polarized LLs using the Lifshitz-Kosevitch formula. By further tracing the LL crossings in the Landau fan diagram, we unambiguously determine the density-dependent valley susceptibility and the interaction enhanced g-factor from 12.7 to 23.6. Near integer ratios of Zeeman-to-cyclotron energies, we discover LL anticrossings due to the formation of quantum Hall Ising ferromagnets, the valley polarizations of which appear to be reversible by tuning the density or an in-plane magnetic field. Our results provide evidence for many-body interaction effects in the conduction band of MoS2 and establish a fertile ground for exploring strongly correlated phenomena of massive Dirac electrons.

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