Journal
JOURNAL OF PHYSICAL CHEMISTRY C
Volume 123, Issue 14, Pages 9364-9370Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.jpcc.9b00228
Keywords
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Funding
- National Natural Science Foundation of China [21661016, 21361012, 21461013]
- Science and Technology Research Project of Jiangxi Provincial Department of Education [GJJ160734]
- Young Scientist Program of Jiangxi Province [20144BCB23038]
- Key Program of Scientific Research of Jinggangshan University [JFD1801]
- Undergraduate Training Programs for Innovation and Entrepreneurship [201810419003]
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Organic-inorganic hybrid metal halides with temperature-triggered responsive switchable dielectric properties have evoked great attention for their potential application in the field of optoelectronic information. Here, we present a new organic-inorganic hybrid metal halide switchable dielectric material, [(C3H5)(2)N(CH3)(2)](2)SnCl6 (1), which is obtained by the reaction of diallyldimethylaminium chloride and tin(IV) chloride pentahydrate. Compound 1 exhibits excellent high-temperature switchable dielectric performance and antifatigue. Notably, 1 also exhibits multifunctionality with semiconducting and photoluminescence property. Such a Sn(IV)-based organic-inorganic hybrid with outstanding switchable dielectric, semiconducting, and photoluminescence characteristics will pave a new approach in the development of Sn(IV)-based metal halides with practical applications.
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