Journal
JOURNAL OF ALLOYS AND COMPOUNDS
Volume 775, Issue -, Pages 342-347Publisher
ELSEVIER SCIENCE SA
DOI: 10.1016/j.jallcom.2018.10.025
Keywords
Solid solutions; Relaxor behavior; Energy density; Na0.5Bi0.5TiO3; BaZrO3
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Funding
- National Natural Science Foundation of China [58172175]
- International Cooperation Projects of Shaanxi Province [2018KW-027]
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Dense (1-x)(0.775NBT-0.225BSN)-xBZ ternary ceramics were fabricated by solid state methods and their dielectric and ferroelectric properties were systematically investigated. XRD and Raman analysis indicate that the structure complexity and phase diffusion were enhanced in 0.775NBT-0.225BSN relaxor system with BZ addition. With increasing the contents of BZ, average grain size greatly decreases. Dielectric study shows that dispersive relaxor-like behavior was beginning to convert to diffusive phase transition when x >= 0.2. Along with increasing the BZ contents, the slop of P-E loops and the energy-loss can gradually decrease. When x = 0.2, both a high W(d )of 2.08 J/cm(3) and eta of 88.8% were achieved, due to the slimer P-E loops, the high P-m(similar to 20 mu C/cm(2)) and E-b(245 kV/cm). As a result, the ternary ceramics system may be a good candidate for energy-storage ceramics of NBT-based materials. (C) 2018 Elsevier B.V. All rights reserved.
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