Journal
ISRAEL JOURNAL OF CHEMISTRY
Volume 59, Issue 9, Pages 832-842Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ijch.201800159
Keywords
Lithium-sulfur batteries; ionic liquids; poly(ionic liquids); Li-metal anode; electrolytes
Categories
Funding
- European Union [666221]
- ARRS Program [P2-0393]
- Max Planck Society
- National Institute of Chemistry (Slovenia)
- University of Munster
- Chalmers University of Technology
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Future optimized lithium-sulfur batteries may promise higher energy densities than the current standard. However, there are many barriers which hinder their commercialization. In this review we describe how ionic liquids (ILs) and their polymers are utilized in different components of the battery to address some of these issues. For example, IL-based electrolytes have the potential to reduce the solubility of polysulfides compared to conventional organic electrolytes. Polymerizing ILs directly on the surface of the Li-metal anode is suggested as an approach to protect the surface of this electrode. Finally, using poly(ionic liquids) (PILs) as binders for the cathode active material may increase the performance of the cathode as compared to polyvinylidene difluoride (PVdF) and could inhibit swelling-induced degradation. These results demonstrate the advantages of ILs and their polymers for improving the performance of Li-S batteries.
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