4.8 Article

Unburned Methane Emissions from Residential Natural Gas Appliances

Journal

ENVIRONMENTAL SCIENCE & TECHNOLOGY
Volume 53, Issue 9, Pages 5473-5482

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.est.8b05323

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Funding

  1. Environmental Defense Fund (EDF)
  2. Alfred P. Sloan Foundation
  3. Brunckhorst Foundation

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Methane, the primary component of natural gas (NG), is a potent greenhouse gas. NG is a common fuel for residential appliances because of low cost, high energy density, and relatively clean combustion. NG exhaust contains some unburned methane due to inevitable incomplete combustion. A field campaign measuring methane concentrations in exhaust from residential NG appliances was conducted in Boston and Indianapolis to determine their contribution to overall emissions. NG space heating, water heating, and cooking appliances were measured in 100 homes. Appliance exhaust typically exhibits a brief methane concentration spike during ignition and extinguishment and relatively low concentrations during steady-state operation. Exceptions to this pattern include ovens, suboptimal stove burners, and tankless water heaters, which either have a different operating pattern or nontrivial steady-state concentrations. Findings were combined with appliance usage and prevalence assumptions to estimate total emissions. Annually, similar to 30 [97.5% CI: 19-160] Gg of methane emissions can be attributed to U.S. residential NG appliances, corresponding to similar to 830 [530-4500] Gg carbon dioxide equivalent (CO(2)e(100)). This accounts for similar to 0.1% [0.08-0.7%] of U.S. anthropogenic methane emissions (which account for similar to 10% of total U.S. greenhouse gas emissions) and corresponds to an emission factor of 0.38 g/kg of NG consumed (0.038% [0.024%-0.21%]).

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