Journal
APPLIED SURFACE SCIENCE
Volume 471, Issue -, Pages 893-899Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.apsusc.2018.11.249
Keywords
Gd-La codoped TiO2 photocatalysts; Liquid phase plasma; Acetaminophen; Band gap energy; Photocatalytic activity
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Funding
- Basic Science Research Program through the National Research Foundation of Korea (NRF) - Ministry of Education [NRF-2018R1D1A1B07049595]
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TiO2 was doped simultaneously with Gd and La using a liquid phase plasma (LPP) reaction to produce a photocatalyst with excellent photoactivity in the visible light region. Gadolinium chloride hexahydrate and lanthanum chloride heptahydrate precursors were used to dope the TiO2 powder with polycrystalline Gd2O3 and La2O3 particles. The doping of TiO2 with rare earth elements using LPP reaction decreased the band gap; the band gap of Gd-La codoped TiO2 photocatalysts (GLTP) was the lowest The photodegradation efficiency of the TiO2 photocatalysts doped with either Gd or La was superior that of bare TiO2 but the photodegradation efficiency of GLTP was highest in both ultraviolet and visible light sources. Acetaminophen (Acetyl-para-aminophen, APAP) was ultimately decomposed to CO2 and H2O via intermediates, such as p-nitrophenol, hydroquinone and hydroxylhydroquinone, by hydroxyl radicals (HO center dot) formed on the surface of GLTP.
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