Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 58, Issue 11, Pages 3594-3598Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201813716
Keywords
2H-pyrans; arylpyridines; dihydropyridines; donor-acceptor cyclopropanes; Heck coupling
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Funding
- DAAD
- DFG [GRK 1910]
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A palladium-catalyzed coupling between aryl halides and monocyclopropanated pyrroles or furans has been developed, leading to valuable six-membered N- and O-heterocycles. As the key step, a selective cleavage of the non-activated endocyclic C-C bond of the 2-heterobicyclo-[3.1.0]hexane framework is achieved. The developed method offers access to highly functionalized piperidines, pyridines, and pyrans that are challenging to access by traditional methods.
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