Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 58, Issue 35, Pages 11978-11996Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201814031
Keywords
Coulombic interaction; electrolytes; interface reactions; rechargeable aluminum batteries
Categories
Funding
- National Natural Science Foundation of China [51525206, 51521091]
- MOST [2016YFA0200100, 2016YFB0100100]
- Strategic Priority Research Program of Chinese Academy of Science [XDA22010602]
- Key Research Program of the Chinese Academy of Sciences [KGZD-EW-T06]
- CAS/SAFEA International Partnership Program
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Aluminum battery systems are considered as a system that could supplement current lithium batteries due to the low cost and high volumetric capacity of aluminum metal, and the high safety of the whole battery system. However, first the use of ionic liquid electrolytes leading to AlCl4- instead of Al3+, the different intercalation reagents, the sluggish solid diffusion process and the fast capacity fading during cycling in aluminum batteries all need to be thoroughly explored. To provide a good understanding of the opportunities and challenges of the newly emerging aluminum batteries, this Review discusses the reaction mechanisms and the difficulties caused by the trivalent reaction medium in electrolytes, electrodes, and electrode-electrolyte interfaces. It is hoped that the Review will stimulate scientists and engineers to develop more reliable aluminum batteries.
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