Journal
ADVANCED SYNTHESIS & CATALYSIS
Volume 361, Issue 8, Pages 1835-1845Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.201801681
Keywords
photoredox; halo-trifluoromethylation; 1; 7-enynes; radical pathway
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Funding
- National Natural Science Foundation of China [21702103, 21522604, U1463201, 21402240]
- Youth in Jiangsu Province Natural Science Fund [BK20150031, BK20130913, BY2014005-03]
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An efficient photoredox-catalyzed halo-trifluoromethylation reaction of 1,7-enynes has been developed under mild conditions. This photocatalytic protocol provides an efficient and functional strategy leading to CF3- and halogen-containing 3,4-dihydroquinolin-2(1H)-ones from a wide range of 1,7-enynes through two different radical pathways. The reaction mechanism was proposed based on the control experiments.
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