Journal
ACS APPLIED MATERIALS & INTERFACES
Volume 11, Issue 17, Pages 15861-15868Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsami.8b21765
Keywords
conjugated microporous polymer; layered architectures; nitrogen and sulfur co-doped; band gap; dye degradation
Funding
- National Natural Science Foundation of China [21875078, 21604028]
- International S&T Cooperation Program of China [2016YFE0124400]
- Program for HUST Interdisciplinary Innovation Team [2016JCTD104]
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Conjugated microporous polymers (CMPs) with high surface areas, tunable building blocks, and fully conjugated structures have found important applications in optoelectronics. Here, we report a new series of CMPs with tunable band gaps by introducing thiazolo[5,4-d] thiazole as the linkage. Because they are synthetic polymers, the geometries and structures could be rationally designed. Their intrinsic wide visible-light absorption properties and layered architectures endow them with a promising photocatalytic performance. The role of geometries, surface areas, and morphologies of the CMPs in photo-catalysis abilities is examined and discussed. The results indicate that geometries have a direct impact on the surface areas and morphologies of the CMPs and thus exert great influence on photocatalysis.
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