Journal
ADVANCED MATERIALS
Volume 28, Issue 12, Pages 2427-2431Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.201505281
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Funding
- National Basic Research Program of China [2015CB932302]
- National Natural Science Foundation of China [21222101, U1432133, 11132009, 21331005, 11321503, U1532265, J1030412, 21173205, 91127042, 11275227, 11179006, 21421063, 21573211]
- Chinese Academy of Sciences [XDB01020000]
- Fok Ying-Tong Education Foundation, China [141042]
- Fundamental Research Funds for the Central Universities [WK2060190027, WK2340000063]
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Isolated single-atom platinum (Pt) embedded in the sub-nanoporosity of 2D g-C3N4 as a new form of co-catalyst is reported. The highly stable single-atom co-catalyst maximizes the atom efficiency and alters the surface trap states of g-C3N4, leading to significantly enhanced photocatalytic H-2 evolution activity, 8.6 times higher than that of Pt nanoparticles and up to 50 times that for bare g-C3N4.
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