Journal
ADVANCED MATERIALS
Volume 28, Issue 43, Pages 9551-+Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.201603401
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Funding
- Natural Scientific Foundation of China [21306103, 21422604, 21561130151]
- Tsinghua University Initiative Scientific Research Program [20161080166]
- Ministry of Science and Technology of the People's Republic of China [2015CB932500, 2016YFA0202500]
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A cooperative interface constructed by lithiophilic nitrogen-doped graphene frameworks and sulfiphilic nickel-iron layered double hydroxides (LDH@NG) is proposed to synergistically afford bifunctional Li and S binding to polysulfides, suppression of polysulfide shuttles, and electrocatalytic activity toward formation of lithium sulfides for high-performance lithium-sulfur batteries. LDH@NG enables high rate capability, long lifespan, and efficient stabilization of both sulfur and lithium electrodes.
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