4.8 Article

High-Performance Integrated Perovskite and Organic Solar Cells with Enhanced Fill Factors and Near-Infrared Harvesting

Journal

ADVANCED MATERIALS
Volume 28, Issue 16, Pages 3159-3165

Publisher

WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.201504555

Keywords

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Funding

  1. National Research Foundation of Korea (NRF) - Korea government (MSIP) [NRF-2014R1A2A1A09006137, NRF-2015K1A3A1A16002247]
  2. R&D program of MSIP/COMPA [2015K000199]
  3. Technology Development Program to Solve Climate Changes of the National Research Foundation (NRF) - Ministry of Science, ICT & Future Planning [NRF-2015M1A2A2057510]
  4. Core Technology Development Program for Next-generation Solar Cells of Research Institute for Solar and Sustainable Energies (RISE), GIST
  5. Ministry of Science, ICT & Future Planning, Republic of Korea [GIST-14] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
  6. National Research Foundation of Korea [2015K1A3A1A16002247, 2015M1A2A2057510, 2014R1A2A1A09006137] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)

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Highly efficient P-I-N type perovskite/bulk-heterojunction (BHJ) integrated solar cells (ISCs) with enhanced fill factor (FF) (approximate to 80%) and high near-infrared harvesting (>30%) are demonstrated by optimizing the BHJ morphology with a novel n-type polymer, N2200, and a new solvent-processing additive. This work proves the feasibility of highly efficient ISCs with panchromatic absorption as a new photovoltaic architecture and provides important design rules for optimizing ISCs.

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