Journal
ADVANCED MATERIALS
Volume 28, Issue 32, Pages 6940-+Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.201601413
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Funding
- National Basic Research Program of China [2015CB932302]
- National Natural Science Foundation of China [U1532265, 21331005, 11321503, 21401181, 91422303, 11404320, 21573211]
- Strategic Priority Research Program of the Chinese Academy of Sciences [XDB01020000]
- Fundamental Research Funds for the Central Universities [WK2060190027, WK2340000063]
- Key Laboratory of Neutron Physics (CAEP) [2014DB01]
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Experimental data reveal that the incorporation of carbonyl groups into polymer matrix can significantly enhance singlet oxygen (O-1(2)) generation and suppress production of other reactive oxygen species. Excitonic processes investigated by phosphorescence spectro scopy reveal enhanced triplet-exciton generation in the modified g-C3N4, which facilitate O-1(2) generation through an energy transfer process. Benefiting from this, the modified g-C3N4 shows excellent conversion and selectivity in organic synthesis.
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