Journal
ADVANCED MATERIALS
Volume 28, Issue 30, Pages 6485-+Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.201601387
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Funding
- National Key Basic Research Program of China [2014CB931801]
- National Natural Science Foundation of China [21475029, 91427302, 51272047]
- Chinese Academy of Sciences [YZ201311, XDA09040100]
- CAS-CSIRO Cooperative Research Program [GJHZ1503]
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A heterogeneous catalyst made of well-defined Co3O4 hexagonal platelets with varied exposed facets is coupled with [Ru(bpy)(3)]Cl-2 photosensitizers to effectively and efficiently reduce CO2 under visible-light irradiation. Systematic investigation based on both experiment and theory discloses that the exposed {112} facets are crucial for activating CO2 molecules, giving rise to significant enhancement of photocatalytic CO2 reduction efficiency.
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