Journal
ADVANCED FUNCTIONAL MATERIALS
Volume 26, Issue 16, Pages 2739-2744Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.201505044
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Funding
- National Basic Research Program of China [2012CB933301]
- National Natural Science Foundation of China [21475064, 61204048]
- Ministry of Education of China [20123223110007]
- Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD)
- Program for Changjiang Scholars and Innovative Research Team in University [IRT_15R37]
- China Postdoctoral Science Foundation [2013M541700]
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Graphene quantum dots (GQDs) with white fluorescence are synthesized by a microwave-assisted hydrothermal method using graphite as the precursor. A solution-processed white-light-emitting diode (WLED) is fabricated using the as-prepared white fluorescent GQDs (white-light-emitting graphene quantum dots, WGQDs) doped 4,4-bis(carbazol-9-yl)biphenyl as the emissive layer. White-light emission is obtained from the WLED with 10 wt% doping concentration of WGQDs, which shows a luminance of 200 cd m(-2) at the applied voltage of 11-14 V. Importantly, an external quantum efficiency of 0.2% is achieved, which is the highest among all the reported WLED based on GQDs or carbon dots. The results demonstrate that WGQDs as a novel phosphor may open up a new avenue to develop the environmentally friendly WLEDs for practical application in solid-state lighting.
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